• Title of article

    Palladium-catalyzed insertion reactions of trimethylsilyldiazomethan

  • Author/Authors

    Kevin L Greenman، نويسنده , , David S Carter، نويسنده , , David L Van Vranken، نويسنده ,

  • Issue Information
    هفته نامه با شماره پیاپی سال 2001
  • Pages
    7
  • From page
    5219
  • To page
    5225
  • Abstract
    Palladium(II) salts catalyze the Kirmse reaction of allylsulfides with trimethylsilyldiazomethane (TMSD) to give homoallylsulfides. Similarly, TMSD can intercept ArPdX intermediates generated during Stille couplings to give benzhydryl derivatives. The yields of this process are limited by overinsertion and β-elimination. Insertion and elimination can be harnessed to generate styrenes from benzylic halides in the presence of palladium (0) catalysts.
  • Keywords
    Insertion , Palladium , carbenes
  • Journal title
    Tetrahedron
  • Serial Year
    2001
  • Journal title
    Tetrahedron
  • Record number

    1082117