• Title of article

    Experimental and QM/MM investigation of the hydrated silica surface reactivity

  • Author/Authors

    Casarin، نويسنده , , Maurizio and Falcomer، نويسنده , , Daniele and Glisenti، نويسنده , , Antonella and Natile، نويسنده , , Marta Maria and Poli، نويسنده , , Fabrizia and Vittadini، نويسنده , , Andrea، نويسنده ,

  • Issue Information
    روزنامه با شماره پیاپی سال 2005
  • Pages
    6
  • From page
    459
  • To page
    464
  • Abstract
    The interaction of a series of molecular probes (O3, H2S, CO, NH3, (CH3)2CO, C5H5N and CH3CN) with the hydrated SiO2 surface has been investigated by QM/MM calculations and diffuse reflectance infrared Fourier transform spectroscopy. Theoretical estimates of O–H stretchings are shown to be improved by a new treatment of the molecular mechanics part of the model. Such a result is encouraging for the application of the adopted approach to other systems.
  • Journal title
    Chemical Physics Letters
  • Serial Year
    2005
  • Journal title
    Chemical Physics Letters
  • Record number

    1915045