DocumentCode
2228650
Title
Electronic coherence effects on population transfer by intense ultrashort chirped pulses in molecules coupled with a dissipative environment
Author
Fainberg, B.D. ; Gorbunov, V.A.
Author_Institution
Dept. of Exact Sci., Holon Acad. Inst. of Technol., Israel
fYear
2002
fDate
19-24 May 2002
Firstpage
216
Abstract
Summary form only given. The effect of relaxation processes on a coherent excitation of a molecule coupled with a dissipative environment is an intriguing question. The purpose of this work is to answer the following question: How does dissipative environment influence on a coherent excitation of a molecule? We have studied the influence of the chirp rate on the excited state population after the completion of pulse action. We used a model of Gaussian-Markovian modulation for description of relaxation processes.
Keywords
Franck-Condon factors; excited states; high-speed optical techniques; molecule-photon collisions; optical pumping; population inversion; Franck-Condon transition; Gaussian-Markovian modulation; dissipative environment coupled molecules; electronic coherence effects; electronic population inversion; excited state population; intense ultrashort chirped pulses; linear chirped pulses; molecule in solution; normalized correlation function; population transfer; population wave; pump-dump process; relaxation processes; saturation parameter; two-level systems; Optical pumping; Ultrafast optics;
fLanguage
English
Publisher
ieee
Conference_Titel
Quantum Electronics and Laser Science Conference, 2002. QELS '02. Technical Digest. Summaries of Papers Presented at the
Conference_Location
Long Beach, CA, USA
Print_ISBN
1-55752-708-3
Type
conf
DOI
10.1109/QELS.2002.1031333
Filename
1031333
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