• DocumentCode
    75516
  • Title

    Planar Laser-Induced Fluorescence Diagnostics for Spatiotemporal OH Evolution in Pulsed Corona Discharge

  • Author

    Chenghang Zheng ; Xu Shen ; Xiang Gao ; Zhongshan Li ; Xinbo Zhu ; Zhongyan Luo ; Kefa Cen

  • Author_Institution
    State Key Lab. of Clean Energy Utilization, Zhejiang Univ., Hangzhou, China
  • Volume
    41
  • Issue
    3
  • fYear
    2013
  • fDate
    Mar-13
  • Firstpage
    485
  • Lastpage
    493
  • Abstract
    OH radicals play an important role in pollutant removal in nonthermal plasmas. It is crucial to clarify the behavior of OH radicals in this process. A time-resolved 2-D OH radial distribution was investigated in a pulsed corona discharge by planar laser-induced fluorescence at atmospheric pressure and room temperature. The OH evolutions under different gas components were studied, and the evolution process was simulated. The OH decay processes were found to be divided into two periods: a fast decay period and a slow decay period. The O, N, and HO2 are dominant radicals for OH generation and decay. The OH radicals are mainly generated near a nozzle electrode. The concentration variations of O2, NO, and H2O in the background gas led to different OH density evolutions. The OH distribution zones were different as gas components varied. The maximum area of OH radical distribution after discharge decreased by 20% as O2 increased from 5% to 8 %, and it decreased by 69% as NO (150 ppm) was added into the background gas.
  • Keywords
    corona; electrodes; fluorescence; free radicals; nitrogen; nitrogen compounds; nozzles; oxygen; oxygen compounds; plasma chemistry; plasma diagnostics; plasma light propagation; plasma simulation; spatiotemporal phenomena; water; H2O; HO2; N; NO; O2; OH; OH decay processes; OH generation; atmospheric pressure; background gas; concentration variations; fast decay period; gas components; nonthermal plasmas; nozzle electrode; planar laser-induced fluorescence diagnostics; pollutant removal; pulsed corona discharge; room temperature; slow decay period; spatiotemporal OH evolution; temperature 293 K to 298 K; time-resolved 2D OH radial distribution; Evolution; OH; planar laser-induced fluorescence (PLIF); pulsed corona discharge;
  • fLanguage
    English
  • Journal_Title
    Plasma Science, IEEE Transactions on
  • Publisher
    ieee
  • ISSN
    0093-3813
  • Type

    jour

  • DOI
    10.1109/TPS.2013.2243919
  • Filename
    6472085