Title of article
Subsystem dynamics in mixed quantum–classical systems Original Research Article
Author/Authors
Mohamad Toutounji، نويسنده , , Raymond Kapral، نويسنده ,
Issue Information
هفته نامه با شماره پیاپی سال 2001
Pages
11
From page
79
To page
89
Abstract
Starting with the mixed quantum–classical Liouville equation, projection operator methods are used to derive an equation of motion for a quantum subsystem dissipatively interacting with a classical bath. The resulting generalized master equation is reduced to the Lindblad equation after making a Markovian approximation in the weak coupling limit. The bath subsystem dynamics is studied from a similar perspective. For situations where the classical subsystem consists of few degrees of freedom, or one is interested in the nature of the modifications of its dynamics as a result of coupling to a large, rapidly relaxing quantum bath, a classical analog of the Lindblad equation is derived and discussed.
Journal title
Chemical Physics
Serial Year
2001
Journal title
Chemical Physics
Record number
1056142
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