• Title of article

    Subsystem dynamics in mixed quantum–classical systems Original Research Article

  • Author/Authors

    Mohamad Toutounji، نويسنده , , Raymond Kapral، نويسنده ,

  • Issue Information
    هفته نامه با شماره پیاپی سال 2001
  • Pages
    11
  • From page
    79
  • To page
    89
  • Abstract
    Starting with the mixed quantum–classical Liouville equation, projection operator methods are used to derive an equation of motion for a quantum subsystem dissipatively interacting with a classical bath. The resulting generalized master equation is reduced to the Lindblad equation after making a Markovian approximation in the weak coupling limit. The bath subsystem dynamics is studied from a similar perspective. For situations where the classical subsystem consists of few degrees of freedom, or one is interested in the nature of the modifications of its dynamics as a result of coupling to a large, rapidly relaxing quantum bath, a classical analog of the Lindblad equation is derived and discussed.
  • Journal title
    Chemical Physics
  • Serial Year
    2001
  • Journal title
    Chemical Physics
  • Record number

    1056142