Migration of minor actinides and lanthanides in fast reactor metallic fuel

Minor actinides (MA) and lanthanides (LA) migration to the cladding in fast reactor metallic fuel is a concern because of their reaction with the cladding material. MA and LA migration test results are analyzed and reactions with the cladding are characterized. Remedies for reducing MA and LA migration and reaction with cladding are reviewed. A possible method is proposed that includes the addition of a compound forming element such as indium or thallium in fuel. These elements preferentially form stable compounds with MA and LA and should therefore reduce migration of MA and LA. As an intrinsic solution to the issue, the feasibility of the use of U–Pu–Mo alloy as fuel is studied. Unlike U–Pu–Zr, U–Pu–Mo consists of a single phase at typical fuel operation temperatures, and should have negligible fuel constituent redistribution and reduce MA and LA migration.