Author/Authors :
Ohtsuki، نويسنده , , Y. and Yahata، نويسنده , , Y. and Kono، نويسنده , , H. and Fujimura، نويسنده , , Y.، نويسنده ,
Abstract :
A locally optimized control theory is developed. This theory is applied to pump–dump laser-driven chemical reactions via an electronically excited state. The results show that the theory can design the pulse shapes for chemical reactions with high quantum yields in strong laser intensity regimes in which perturbative treatments break down.
