Author/Authors :
Nakano، نويسنده , , Masayoshi and Matsuzaki، نويسنده , , Yoichi and Nagao، نويسنده , , Hidemi and Yamada، نويسنده , , Satoru and Shigemoto، نويسنده , , Isamu and Yamaguchi، نويسنده , , Kizashi، نويسنده ,
Abstract :
A method is developed for a nonperturbative calculation of nonlinear optical susceptibilities for specific systems such as low-density gases or single molecule systems, including effects of nuclear motion. Nuclear motion is treated quantum-mechanically by wave packet dynamics with population damping effects. As an example, the effects of temperature and mass on the third-order susceptibilities for a three-atom cation model system are examined.
