Author/Authors :
Grنfe، نويسنده , , Stefanie and Marquetand، نويسنده , , Philipp and Engel، نويسنده , , Volker and Henriksen، نويسنده , , Niels E. and Mّller، نويسنده , , Klaus B.، نويسنده ,
Abstract :
We derive electric fields for the purpose of controlling molecular processes taking the instantaneous dynamics of the molecule into consideration. In this way, it is not only possible to achieve a highly efficient control but, more importantly, to give the derived fields a clear physical interpretation. The scheme is illustrated for the cases of excited state IR dissociation of NaI and for a proton-transfer process, treated within a simplified model.