Author/Authors :
Thorwart، نويسنده , , M. and Eckel، نويسنده , , J. and Reina، نويسنده , , J.H. and Nalbach، نويسنده , , P. and Weiss، نويسنده , , S.، نويسنده ,
Abstract :
We show that quantum coherence of biomolecular excitons is maintained over exceedingly long times due to the constructive role of their non-Markovian protein-solvent environment. Using a numerically exact approach, we demonstrate that a slow quantum bath helps to sustain quantum entanglement of two pairs of Fِrster coupled excitons, in contrast to a Markovian environment. We consider the cross-over from a fast to a slow bath and from weak to strong dissipation and show that a slow bath can generate robust entanglement. This persists to surprisingly high temperatures, even higher than the excitonic gap and is absent for a Markovian bath.