Optically-induced molecular reorientation in nematic liquid crystals and nonlinear optical processes in the nanoseconds regime

We present a detailed theoretical analysis and experimental study of purely optically-induced nematic axis reorientation and the associated nonlinear optical processes such as self-phase modulations and optical switching. It is shown that under a sufficiently intense laser field (∼ 100 MW/cm²), nematic liquid crystals will respond in the nanosecond regime. Single nanosecond laser pulse self-phase modulation and intensity switching effects are observed. The magnitude and dynamics of the response are in agreement with theoretical expectations. Optical power limiting and switching effects associated with self-phase modulations are also demonstrated.