Title :
Frequency-Dependent Complex Conductivities and Dielectric Responses of Indium Tin Oxide Thin Films From the Visible to the Far-Infrared
Author :
Chen, Ching-Wei ; Lin, Yen-Cheng ; Chang, Chia-Hua ; Yu, Peichen ; Shieh, Jia-Min ; Pan, Ci-Ling
Author_Institution :
Dept. of Photonics, Nat. Chiao Tung Univ., Hsinchu, Taiwan
Abstract :
Transparent and conducting indium tin oxide (ITO) thin films form an integral part for various optoelectronic devices. In this paper, we report the frequency-dependent complex conductivities and dielectric responses of several sputtered ITO thin films with thicknesses in the range of 189-962 nm by using terahertz time domain spectroscopy (THz-TDS), optical reflectance spectroscopy, and electrical measurements. The plasma frequencies are verified to be from 1590 to 1930 rad·THz, while the scattering times are in the range 6-7 fs based on the Drude free-electron model. The mobilities of the above ITO thin films are calculated to be 32.7-34.2 cm2 V-1 s-1, whereas the carrier concentrations lie in the range 2.79-4.10× 1020 cm-3. The electrical properties derived from the THz-TDS technique agree well with those determined by Hall measurement. Parameters for the complex dielectric function suitable for ITO in the range 0.2-2 and 4-450 THz are also determined.
Keywords :
Hall mobility; dielectric function; electrical conductivity measurement; electron density; high-frequency effects; indium compounds; infrared spectra; optical films; optical time-domain reflectometry; semiconductor growth; semiconductor plasma; semiconductor thin films; sputter deposition; terahertz wave spectra; transparency; visible spectra; wide band gap semiconductors; Drude free-electron model; Hall measurement; ITO; carrier concentration; carrier mobility; complex dielectric function; electrical measurement; frequency 0.2 THz to 2 THz; frequency 4 THz to 450 THz; frequency-dependent complex conductivity; infrared spectra; optical reflectance spectroscopy; plasma frequency; reactive magnetron sputtering; size 189 nm to 962 nm; terahertz time domain spectroscopy; transparent indium tin oxide thin films; visible spectra; wide-bandgap semiconductor; Conductivity; Dielectrics; Indium tin oxide; Optical films; Refractive index; Substrates; Time frequency analysis; Dielectric function; drude free-electron model; indium tin oxide; optical constants; plasma frequency; scattering time; terahertz time domain spectroscopy;
Journal_Title :
Quantum Electronics, IEEE Journal of
DOI :
10.1109/JQE.2010.2063696