DocumentCode :
1517883
Title :
A New Scintillator for Fast Neutron Detection: Single-Crystal {\\rm CeCl}_{3}({\\rm CH}_{3}{\\rm OH})_{4}
Author :
Neal, J.S. ; Boatner, L.A. ; Bell, Z.W. ; McConchie, S.M. ; Wisniewski, D. ; Ramey, J.O. ; Kolopus, J.A. ; Chakoumakos, B.C. ; Wisniewska, M. ; Custelcean, R.
Author_Institution :
Center for Radiat. Detection Mater. & Syst., Oak Ridge Nat. Lab., Oak Ridge, TN, USA
Volume :
57
Issue :
3
fYear :
2010
fDate :
6/1/2010 12:00:00 AM
Firstpage :
1692
Lastpage :
1696
Abstract :
A new scintillator material for the detection of fast neutrons that consists of a methanol adduct of cerium trichloride with the composition CeCl3(CH3OH)4 has been characterized using 14.1 MeV neutrons from a deuterium-tritium neutron generator and fast neutrons from a bare instrumented 252Cf source. The timing resolution of the scintillator for fast neutrons was found to be 1~ ns. Neutron interactions in the CeCl3(CH3OH)4 composition were simulated using the MCNP-PoliMi code. These simulations indicate that proton recoils account for most of the deposited energy in CeCl3(CH3OH)4. The crystalline molecular adduct CeCl3(CH3OH)4 represents a rare-earth metal-organic scintillator that can be applied to both fast neutron and gamma-ray detection.
Keywords :
gamma-ray detection; neutron detection; organic compounds; solid scintillation detectors; 252Cf source; MCNP-PoliMi code; cerium trichloride; crystalline molecular adduct; deposited energy; deuterium-tritium neutron generator; fast neutron detection; gamma-ray detection; neutron interactions; rare-earth metal-organic scintillator; scintillator material; scintillator timing resolution; single-crystal CeCl3(CH3OH)4; Cerium; Character generation; Composite materials; Crystallization; Gamma ray detection; Instruments; Methanol; Neutrons; Protons; Timing; Fast neutron; metal organic; rare earth; scintillator;
fLanguage :
English
Journal_Title :
Nuclear Science, IEEE Transactions on
Publisher :
ieee
ISSN :
0018-9499
Type :
jour
DOI :
10.1109/TNS.2010.2046911
Filename :
5485147
Link To Document :
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