Title :
Femtosecond two-dimensional Fourier transform electronic spectroscopy
Author :
Yetzbacher, Michael K. ; Smith, Eric Ryan ; Cho, Byungmoon ; Kitney, Katherine A. ; Jonas, David M.
Author_Institution :
Dept. of Chem. & Biochem., Colorado Univ., Boulder, CO
Abstract :
Two-dimensional spectra are obtained by Fourier transformation of four-wave mixing signal fields with respect to time delays between femtosecond pulses. We discuss peak shapes, experimental distortions, and dispersion relations. Two-dimensional electronic spectra revealing solvent and electronic motion are used as illustrations.
Keywords :
Fourier transform spectroscopy; high-speed optical techniques; multiwave mixing; two-dimensional spectroscopy; Fourier transformation; dispersion relations; electronic motion; femtosecond 2D Fourier transform electronic spectroscopy; femtosecond pulses; four-wave mixing signal fields; solvent motion; Dispersion; Fourier transforms; Frequency; Optical distortion; Optical pulses; Optical refraction; Signal resolution; Spectroscopy; Ultrafast electronics; Ultrafast optics;
Conference_Titel :
Lasers and Electro-Optics - Pacific Rim, 2007. CLEO/Pacific Rim 2007. Conference on
Conference_Location :
Seoul
Print_ISBN :
978-1-4244-1173-3
Electronic_ISBN :
978-1-4244-1174-0
DOI :
10.1109/CLEOPR.2007.4391235
