DocumentCode :
2536635
Title :
Construction of an ESR-STM for single molecular based magnets anchored at surfaces
Author :
Messina, Paolo ; Sigalotti, Paolo ; Lenci, Lorenzo ; Prato, Stefano ; Gatteschi, Dante
Author_Institution :
INSTM Unita´´ di Firenze, Sesto Fiorentino, Italy
fYear :
2004
fDate :
16-19 Aug. 2004
Firstpage :
642
Lastpage :
644
Abstract :
Reading and manipulating the spin status of single magnetic molecules is of paramount importance both for applicative and fundamental purposes. The possibility to combine electron spin resonance (ESR) and scanning tunnelling microscopy (STM) has been explored one decade ago. A few experiments have raised the question whether or not an EPR spectrum of single molecule is detachable. Only a few data have been reported in modern surface science literature. To date it has yet to be proven till which extent ESR can be reliably and reproducibly performed on single molecules. We are setting up a new ESR-STM "spectrometer" to verify and study the effect of spin-spin correlations in the frequency spectrum of the tunneling current which flows through a single magnetic adsorbate and a metal surface. Here, we discuss, the major experimental challenges that we are attempting to overcome.
Keywords :
EPR spectrometers; magnetic tunnelling; molecular magnetism; scanning tunnelling microscopy; spin-spin interactions; EPR spectrum; ESR-STM spectrometer; electron spin resonance; frequency spectrum; metal surface; scanning tunnelling microscopy; single magnetic adsorbates; single molecular based magnets; spin status; spin-spin correlations; tunneling current; Instruments; Magnetic field measurement; Magnetic fields; Magnetic resonance; Magnets; Molecular electronics; Paramagnetic resonance; Radio frequency; Signal design; Tunneling;
fLanguage :
English
Publisher :
ieee
Conference_Titel :
Nanotechnology, 2004. 4th IEEE Conference on
Print_ISBN :
0-7803-8536-5
Type :
conf
DOI :
10.1109/NANO.2004.1392446
Filename :
1392446
Link To Document :
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