Squeezing of a one-dimensional phonon in a halogen-bridged mixed-valence metal complex

Author

Misawa, K. ; Sugita, A. ; Janszky, J. ; Yamashita, M. ; Kobayashi, T.

Author_Institution

Dept. of Phys., Tokyo Univ., Japan

fYear

1992

fDate

23-28 May 1992

Firstpage

165

Abstract

Summary form only given. Recent progress of femtosecond lasers has enabled us to observe real-time dynamics of nuclear motions in molecular systems. Moreover, quantum control of vibrational wavepackets is one of the most exciting subjects, because the products of chemical reactions can be selected by means of wavepacket shaping using tailored femtosecond pulses. We discuss the generation of the squeezed phonons associated with one-dimensional excitons in a mixed-valence metal complex. The present study is the first observation of the vibrational squeezing of the Franck Condon states in condensed matters.

Keywords

Franck-Condon factors; high-speed optical techniques; optical squeezing; phonons; vibrational states; 1D excitons; Franck Condon states; chemical reactions; condensed matter; femtosecond lasers; halogen-bridged mixed-valence metal complex; mixed-valence metal complex; molecular systems; nuclear motions; one-dimensional excitons; one-dimensional phonon squeezing; real-time dynamics; squeezed phonon generation; tailored femtosecond pulses; vibrational squeezing; vibrational wavepackets; wavepacket shaping; Chemical lasers; Excitons; Laser theory; Motion control; Phonons; Physics; Pulse amplifiers; Pulse measurements; Real time systems; Shape control;

fLanguage

English

Publisher

ieee

Conference_Titel

Quantum Electronics and Laser Science Conference, 1999. QELS '99. Technical Digest. Summaries of Papers Presented at the

Conference_Location

Baltimore, MD, USA

Print_ISBN

1-55752-576-X

Type

conf

DOI

10.1109/QELS.1999.807475

Filename

807475