Title :
Electron transfer between quasi-zero-dimensional nanostructures
Author :
Karel Král;Miroslav Menŝík
Author_Institution :
Institute of Physics, Academy of Sciences of Czech Republic, v.v.i. Na Slovance 2,18221 Prague, Czech Republic
Abstract :
The electric charge transport is an important phenomenon in the systems like interacting quantum dots and molecules, and in polymers, including DNA molecules. We expect that in these nanostructure systems the key role is played by the interaction of the charge carriers with the optical phonons. We show the role of the multiple scattering of the charge carriers on the optical phonons in the inter-molecular transfer. The charge carrier transport based on this mechanism will be discussed theoretically and compared with the earlier experimental results on the charge transport in molecular Donor-Acceptor charge transfer crystals and also in other systems. In order to treat theoretically the electron transfer between two zero-dimensional nanostructures, we will use for simplicity the model of two interacting quantum dots coupled by the electron inter-dot tunneling mechanism. A connection with the popular Marcus semiclassical charge transfer theory, between two quasi-zero-dimensional reactants in chemistry, is also shown. We will use the nonequilibrium quantum electronic transport theory based on the nonequilibrium Green´s functions.
Keywords :
"Nanostructures","Charge carriers","Optical scattering","Quantum dots","Electron optics","Optical polymers","Phonons","Charge transfer","Quantum mechanics","DNA"
Conference_Titel :
Transparent Optical Networks (ICTON), 2010 12th International Conference on
Print_ISBN :
978-1-4244-7799-9
DOI :
10.1109/ICTON.2010.5548991