DocumentCode
405412
Title
Investigation of sum-frequency generation of chiral molecules in solutions
Author
Hayashi, M. ; Lin, S.H. ; Shen, Y.R.
Author_Institution
Center for Condensed Matter Sci., Nat. Taiwan Univ., Taiwan
Volume
1
fYear
2003
fDate
15-19 Dec. 2003
Abstract
A main purpose of this paper is to examine the origin and mechanism of nonlinear optical activity in solution. For this purpose, within the dipole-dipole formalism of SFG, we study the nonCondon effect and the effect of the breakdown of the Born-Oppenheimer approximation. We find that in order to determine which mechanism is responsible for this SFG it is necessary to compare the SFG band-shape functions on surfaces and in solutions.
Keywords
chirality; magnetic moments; optical frequency conversion; Born-Oppenheimer approximation; SFG; band-shape functions; chiral molecules; dipole-dipole formalism; nonCondon effect; nonlinear optical activity; sum-frequency generation; Art; Atom optics; Electric breakdown; Frequency; Laboratories; Nonlinear optics; Optical materials; Physics; Signal generators;
fLanguage
English
Publisher
ieee
Conference_Titel
Lasers and Electro-Optics, 2003. CLEO/Pacific Rim 2003. The 5th Pacific Rim Conference on
Print_ISBN
0-7803-7766-4
Type
conf
DOI
10.1109/CLEOPR.2003.1274645
Filename
1274645
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