Title :
Crystal Growth and Scintillation Properties of 2-Inch-Diameter
(Pr:LuAG) Single Crystal
Author :
Kamada, Kei ; Tsutsumi, Kousuke ; Usuki, Yoshiyuki ; Ogino, Hiraku ; Yanagida, Takayuki ; Yoshikawa, Akira
Author_Institution :
Mater. Res. Lab., Furukawa Co. Ltd., Tsukuba
fDate :
6/1/2008 12:00:00 AM
Abstract :
In this work we tried to grow 2-inch-diameter and high quality Pr:LuAG single crystals by the Czochralski (Cz) method. To grow the large diameter Pr:LuAG single crystal, we have optimized growth conditions and the furnace design. As a result, we have succeeded in the growth of 2-inch-diameter Pr:LuAG single crystal with a length of 110 mm. To determine light yield and energy resolution the energy spectra were collected under 662 keV gamma-ray excitation (137Cs source) and detection by a photomultiplier (Hamamatsu H7826). The light yield was around three times higher than that of BGO and almost homogeneous with increasing solidification fraction up to 0.32. The energy resolution was around 8%. Furthermore, scintillation decay time was around 23 ns and almost homogeneous all over the crystal.
Keywords :
crystal growth from melt; gamma-ray detection; gamma-ray effects; lutetium compounds; photoluminescence; photomultipliers; praseodymium; scintillation counters; solidification; 5d-4f luminescence; Czochralski method; Lu3Al5O12:Pr; Pr:LuAG single crystal; Pr3+; crystal growth; electron volt energy 662 keV; energy spectra; gamma-ray detectors; gamma-ray effects; garnets; photoluminescence; photomultiplier; scintillation decay time; scintillation properties; size 110 mm; size 2 in; solidification; Automatic control; Chemical analysis; Control systems; Crystalline materials; Crystals; Design optimization; Energy resolution; Materials science and technology; Performance analysis; Time measurement; 5d-4f luminescence; ${rm Pr}^{3+}$; crystal growth; gamma-ray detectors; garnets;
Journal_Title :
Nuclear Science, IEEE Transactions on
DOI :
10.1109/TNS.2008.924072