Title :
A Ceramic Version of the LSO Scintillator
Author :
Lempicki, A. ; Brecher, C. ; Lingertat, H. ; Miller, S.R. ; Glodo, J. ; Sarin, V.K.
Author_Institution :
ALEM Assoc., Boston, MA
fDate :
6/1/2008 12:00:00 AM
Abstract :
Although LSO is one of the most successful scintillator developments for medical diagnostics in the last two decades, good single crystals are not commercially available in any quantity. Consequently, we explored the feasibility of developing a ceramic version of the material, which requires a considerably lower temperature to consolidate the material to essentially crystalline density. Consolidation of the ceramic was achieved by hot pressing at temperatures up to 1700degC and pressure of 8000 psi. Hot pressing causes a loss of oxygen resulting in strong coloration of the ceramic, which had to be removed by heating (ldquobleachingrdquo) in air at approximately 1100degC. The resultant specimens were colorless and highly translucent, but the anisotropic nature of the crystal structure precluded the achievement of full transparency. The scintillation performance of the resulting ceramics was characterized and compared with that of high light-output LSO single crystals. The scintillation efficiency as measured by energy spectra generally fell in the range of 50-60% of that of the crystals. While this would be adequate for PET applications, the limited transparency provides a barrier to such use. An alternative application would be in signal integrating techniques, such as CT, where it could provide an alternative to GOS but with higher speed. Here, the problem of afterglow assumes major importance. The afterglow is a function of many factors, including conditions of excitation. Further work on improving the LSO ceramics is considered.
Keywords :
ceramics; crystal structure; doping; hot pressing; lutetium compounds; positron emission tomography; scintillation; scintillation counters; silicon compounds; LSO ceramics; LSO scintillators; Lu2OSiO4:Ce; PET applications; afterglow; ceramic scintillators; crystal structure; crystalline density; energy spectra; hot pressing; light-output LSO single crystals; medical diagnostics; scintillation efficiency; signal integrating techniques; temperature 1100 C; temperature 1700 C; Anisotropic magnetoresistance; Bioceramics; Ceramics; Crystalline materials; Crystallization; Crystals; Heating; Medical diagnosis; Pressing; Temperature; Afterglow; LSO; ceramic scintillators; efficiency; transparency;
Journal_Title :
Nuclear Science, IEEE Transactions on
DOI :
10.1109/TNS.2007.914368